摘要
Sustainable energy supplies are needed to supplement and eventually replace fossil fuels. Molecular hydrogen H2 is a clean burning, high-energy fuel that is also used as reducing gas in industrial processes. H2 is mainly synthesized by steam reforming of natural gas, a non-renewable fuel. There are biosynthetic strategies for H2 production; however, they are associated with poor yield and have high cost. The application of an electrochemical driving force in a microbial electrolysis cell (MEC) improves the yield of biological reactions. The performance of the MEC is influenced by experimental parameters such as the electrode material, reactor design, microbial consortia and the substrate. In this review, factors that affect the performance of MECs are discussed and critically analysed. The potential for scale-up of H2 bioelectrosynthesis is also discussed.
摘要译文
需要可持续能源来补充和最终取代化石燃料。分子氢H 2是一种清洁燃烧的高能燃料,也被用作工业过程中的还原气体.H 2主要是通过天然气蒸汽重整,不可再生燃料。H 2生产有生物合成策略;然而,它们的产率低,成本高。微生物电解池(MEC)中电化学驱动力的应用提高了生物反应的产率.MEC的性能受实验参数的影响,如电极材料,反应器设计,微生物联合体和底物。在此综述中,对影响MECs性能的因素进行了讨论和批判性分析。还讨论了H 2生物电合成扩大的潜力
Michael Kitching[a]; Robin Butler[a]; Enrico Marsili[b]. Microbial bioelectrosynthesis of hydrogen: Current challenges and scale-up[J]. Enzyme and Microbial Technology, 2017,96: 1–13